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Mechanism insight into rapid photocatalytic disinfection of Salmonella based on vanadate QDs-interspersed g-C3N4 heterostructures
Wang, Rong ; Kong, Xiangyu ; Zhang, Wentao ; Zhu, Wenxin ; Huang, Lunjie ; Wang, Jing ; Zhang, Xu ; Liu, Xinnan ; Hu, Na ; Suo, Yourui ; Wang, Jianlong
2018-06-05
发表期刊APPLIED CATALYSIS B-ENVIRONMENTAL
摘要Photocatalytic disinfection, which is a readily reliable method in most climates, holds great promise to significantly reduce the microbial contamination in modern industry. Here we report that vanadate quantum dots interspersed graphitic carbon nitride (vanadate QDs/g-C3N4) can achieve efficient inactivation of Salmonella by harvesting a substantial visible light. Detailed characterization through SEM-EDS, TEM, XRD, FT-IR, and XPS confirmed the formation of the composites. Owing to the efficient reactive oxygen species (ROS) production between vanadate QDs and g-C3N4, the bactericidal efficiency of AgVO3 QDs/g-C3N4 could reach 96.4% toward Salmonella in a concentration of 0.75 mg/mL after 10 min visible-light illumination. More importantly, scavenger experiments, of different reactive species proved that the photoinduced electron generated at the oxidation site of AgVO3/g-C3N4 play a major role as oxidative species. Fluorescent-based cell live/dead test and membrane potentials were applied to demonstrate the integrity of cell membranes. Furthermore, the SEM technology, PCR and BCA protein assay were employed to verify the bacterial decomposition as well as leakage of bacterial cell contents toward Salmonella. Sterilization experiments of Staphylococcus auteus revealed that our composites have broad spectrum antimicrobial activity for both Gram-negative and Gram-positive bacteria under visible light. The results showed that the generation of high ROS could attack the bacterial cells membrane, and ultimately disrupt the cell metabolism through bacterial contents, which provided a feasible method for eliminating the microbial contaminated water.
文献类型期刊论文
条目标识符http://210.75.249.4/handle/363003/49269
专题中国科学院西北高原生物研究所
推荐引用方式
GB/T 7714
Wang, Rong,Kong, Xiangyu,Zhang, Wentao,et al. Mechanism insight into rapid photocatalytic disinfection of Salmonella based on vanadate QDs-interspersed g-C3N4 heterostructures[J]. APPLIED CATALYSIS B-ENVIRONMENTAL,2018.
APA Wang, Rong.,Kong, Xiangyu.,Zhang, Wentao.,Zhu, Wenxin.,Huang, Lunjie.,...&Wang, Jianlong.(2018).Mechanism insight into rapid photocatalytic disinfection of Salmonella based on vanadate QDs-interspersed g-C3N4 heterostructures.APPLIED CATALYSIS B-ENVIRONMENTAL.
MLA Wang, Rong,et al."Mechanism insight into rapid photocatalytic disinfection of Salmonella based on vanadate QDs-interspersed g-C3N4 heterostructures".APPLIED CATALYSIS B-ENVIRONMENTAL (2018).
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