Knowledge Management System of Northwest Institute of Plateau Biology, CAS
Mechanism investigation for ultra-efficient photocatalytic water disinfection based on rational design of indirect Z-scheme heterojunction black phosphorus QDs/Cu2O nanoparticles | |
Luo, SJ; Liu, RX; Zhang, XX; Chen, R; Yan, MM; Huang, KR; Sun, J; Wang, R; Wang, JL | |
2022 | |
发表期刊 | JOURNAL OF HAZARDOUS MATERIALS |
卷号 | 424 |
摘要 | Photocatalysis has been regarded as a promising inactivation technology targeting to reduce drug-resistant bacteria contamination, but developing efficient photocatalysts with broad visible light harvesting capability is still a challenge. Here we report a MOFs-derived BPQDs/Cu2O/N-doped hollow porous carbon (BP/CNC) with indirect Z-scheme heterojunctions (BPQDs/Cu2O), which can inactivate 99.99999% Methicillin-resistant Staphylococcus aureus (MRSA) at a concentration of only 10 mg/L. Combining photoelectrochemical techniques and electrochemical measurements, the efficient inactivation process was attributed to the synergistic effect of enhanced light utilization and effective suppression of photogenerated carrier recombination. The mechanism of gradually damaged cell membrane for MRSA was studied by employing scanning electron microscopy (SEM), fluorescence staining and coagulase titer test to further decipher the changes in bacterial cells. We propose that reactive oxygen species (ROS) destroys the cell wall membrane and causes the leakage of cell contents, eventually leading to death. In addition, a series of in vitro and in vivo toxicity tests were conducted to evaluate the biocompatibility of the antibacterial system and its potential use in practice. This strategy of BPQDs/ Cu2O indirect heterojunction fabrication can spatially inhibit the recombination of photogenerated carriers, expands the light absorption range, providing a feasible method for disinfecting microbial contaminated water. |
收录类别 | SCIE |
文献类型 | 期刊论文 |
条目标识符 | http://210.75.249.4/handle/363003/61364 |
专题 | 中国科学院西北高原生物研究所 |
推荐引用方式 GB/T 7714 | Luo, SJ,Liu, RX,Zhang, XX,et al. Mechanism investigation for ultra-efficient photocatalytic water disinfection based on rational design of indirect Z-scheme heterojunction black phosphorus QDs/Cu2O nanoparticles[J]. JOURNAL OF HAZARDOUS MATERIALS,2022,424. |
APA | Luo, SJ.,Liu, RX.,Zhang, XX.,Chen, R.,Yan, MM.,...&Wang, JL.(2022).Mechanism investigation for ultra-efficient photocatalytic water disinfection based on rational design of indirect Z-scheme heterojunction black phosphorus QDs/Cu2O nanoparticles.JOURNAL OF HAZARDOUS MATERIALS,424. |
MLA | Luo, SJ,et al."Mechanism investigation for ultra-efficient photocatalytic water disinfection based on rational design of indirect Z-scheme heterojunction black phosphorus QDs/Cu2O nanoparticles".JOURNAL OF HAZARDOUS MATERIALS 424(2022). |
条目包含的文件 | 条目无相关文件。 |
除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。
修改评论