Knowledge Management System of Northwest Institute of Plateau Biology, CAS
Fixed-bed column studies for the removal of anionic dye from aqueous solution using TiO2@glucose carbon composites and bed regeneration study | |
Zheng, Pei1; Bai, Bo3; Guan, Weisheng1; Wang, Honglun2; Suo, Yourui2 | |
2016 | |
发表期刊 | JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS
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卷号 | 27期号:1页码:867-877 |
文章类型 | Article |
摘要 | Glucose carbon with uniform diameter was successfully anchored by TiO2 nanoparticles via a facile low-temperature hydrothermal process independent of surfactants or external forces. The resultant TiO2@glucose carbon composite (TiO2@GCs) was characterized by scanning electron microscopy (SEM) and energy dispersive spectrometry (EDS). The elimination of direct deep blue (DDB) from aqueous solution by adsorption onto TiO2@GCs was investigated in the up-flow fixed-bed columns. The effects of the influent concentration (10-30 mg L-1), flow rate (3-5 mL min(-1)), bed depth (1.0-2.0 cm) and pH (1.0-9.0) were investigated. Breakthrough time and adsorption capacity of the fixed-bed increased with increasing bed depth, whereas decreased with the increase in initial concentration, bed depth and solution pH values. The experimental data was in good agreement with both Thomas model and Yoon-Nelson model. The employed bed saturated with DDB was readily regenerated through a simple regeneration process with UV irradiation for 1 h. Furthermore, the adsorption-regeneration process was conducted for six cycles and no major decrease of regeneration efficiency was observed for the first three cycles. One possible mechanism for regenerating dye-loaded TiO2@GCs was proposed. The verifying experiment found that hydroxyl radicals and superoxide ions significantly affected the regeneration of employed TiO2@GCs bed. |
WOS标题词 | Science & Technology ; Technology ; Physical Sciences |
DOI | 10.1007/s10854-015-3828-z |
关键词[WOS] | METHYLENE-BLUE ; RICE HUSK ; ADSORPTION ; DEGRADATION ; WASTE ; BIOSORPTION ; ADSORBENT ; OXIDATION ; KINETICS ; BATCH |
收录类别 | SCI |
语种 | 英语 |
项目资助者 | National Natural Science Foundation of China(21176031) ; Shanxi Provincial Natural Science Foundation of China(2015JM2071) ; Fundamental Research Funds for the Central Universities-A Foundation for the Author of Excellent Doctoral Dissertation of Chang'an University(310829150004) ; Fundamental Research Funds for the Central Universities(310829151073) |
WOS研究方向 | Engineering ; Materials Science ; Physics |
WOS类目 | Engineering, Electrical & Electronic ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter |
WOS记录号 | WOS:000368054600114 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://210.75.249.4/handle/363003/6499 |
专题 | 中国科学院西北高原生物研究所 |
作者单位 | 1.Changan Univ, Coll Environm Sci & Engn, Xian 710054, Peoples R China 2.Chinese Acad Sci, Northwest Plateau Inst Biol, Xining 810001, Peoples R China 3.Chinese Acad Sci, Northwest Plateau Inst Biol, Key Lab Tibetan Med Res, Xining 810001, Peoples R China |
推荐引用方式 GB/T 7714 | Zheng, Pei,Bai, Bo,Guan, Weisheng,et al. Fixed-bed column studies for the removal of anionic dye from aqueous solution using TiO2@glucose carbon composites and bed regeneration study[J]. JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS,2016,27(1):867-877. |
APA | Zheng, Pei,Bai, Bo,Guan, Weisheng,Wang, Honglun,&Suo, Yourui.(2016).Fixed-bed column studies for the removal of anionic dye from aqueous solution using TiO2@glucose carbon composites and bed regeneration study.JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS,27(1),867-877. |
MLA | Zheng, Pei,et al."Fixed-bed column studies for the removal of anionic dye from aqueous solution using TiO2@glucose carbon composites and bed regeneration study".JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS 27.1(2016):867-877. |
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